Selective IR absorption in molecular nanofilms

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dc.citation.epage1584
dc.citation.spage1578
dc.citation.volume33
dc.contributor.authorŠkipina, B.
dc.contributor.authorMirjanić, D. Lj.
dc.contributor.authorVučenović, S. M.
dc.contributor.authorŠetrajčić, J. P.
dc.contributor.authorŠetrajčić, I. J.
dc.contributor.authorŠetrajčić-Tomić, A. J.
dc.contributor.authorPelemiš, S. S.
dc.contributor.authorMarkoski, B.
dc.date.accessioned2023-09-14T12:05:27Z
dc.date.available2023-09-14T12:05:27Z
dc.date.issued2011
dc.description.abstractWe have formulated a microscopic theory of optical properties of ultrathin molecular films (nanofilms), i.e. quasi 2D systems parallel to XY planes bounded by two surfaces. Exposure of nanofilms to the external electromagnetic fields has result in creation of excitons – but different than bulk ones. Harmonic exciton states were calculated using the method of two-time, retarded, temperature dependent Green’s functions. It has been shown that two types of optical excitations can occur: bulk and surface exciton states. Exciton energy dispersion law shows discrete behavior with non-zero values. Analysis of the dielectric properties of these crystalline systems for low exciton concentration shows that the permittivity strongly depends on boundary parameters and the thickness of the film. In addition, permittivity shows very narrow and discrete dependence of external electromagnetic field frequency, which is a consequence of both resonance and quantum size effects. Influences of boundary conditions on optical characteristics (through analyses of dynamical absorption coefficient) of these nanostructures were specially and in details explored.
dc.identifier.urihttps://vaseljena.ues.rs.ba/handle/123456789/768
dc.language.isoen
dc.publisherElsevier
dc.sourceOptical Materials
dc.subjectNanofilm, Excitons, Permittivity, Absorption index, Green’s functions
dc.titleSelective IR absorption in molecular nanofilms
dc.typeArticle
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